Yeah, I love watching old TV shows (from the 4:3 era) on a CRT TV the way I watched them when they originally aired. I think they look great, and it adds to the nostalgia for me. I use that same 32" CRT TV for playing classic video games too, mostly Atari 2600, NES, and SNES.
I like watching things the way they were originally intended to be seen, or as close to it as I can realistically get, so when it comes to Hollywood movies, I stick with Blu-rays and watch them on a 1080p DLP projector, which approximates the resolution of a 35mm release print (35mm camera negatives can resolve to around 4K, but the release prints shown in theaters had several generations of loss compared to those). Since all my favorite movies are pretty old now, they were all shot on 35mm film and originally shown on film projectors in theaters. Owning a 35mm film projector and collecting gray-market 35mm release prints is for rich people, not for me, but I'm happy with the results of Blu-rays, my projector, and a 100" screen in my living room. The essence is still there, i.e., a projected image like in a theater; reflected light rather than looking at a light source as you do with a direct-view display.
I'm having a blast with these TNG DVDs. I haven't watched TNG since its original run (which started when I was 12 years old), and I'd forgotten how good some of the episodes are. We only got perfect reception on channel 5, and unfortunately, TNG (and TOS reruns too) aired on channel 7, which we only got about 90% reception on at best, and usually more like 75%, so watching these on DVD gives me the perfect reception I wished for when I was a kid.